Cryptic crossword clue
Besotted with slinky demeanour 9

The most common and most likely answer to this crossword clue is the 9 letter word ENAMOURED

I've seen this crossword clue in The Times
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Buddy explains!

The straight part
We know that "Besotted" is the straight/definition part of the clue. The straight part is often a synonym or definition, in this case besotted = enamoured.
The cryptic/wordplay part
In cryptic crossword there's often an wordplay/cryptic part as well.
This part involves a more complex hint, such as an anagram, homophone, hidden word, etc.
Sadly, We don't have an explanation for this specific crossword clue yet.

What does ENAMOURED mean?

ENAMOURED verb
  1. (mostly in the passive, followed by "of" or "with") To cause to be in love.
  2. (mostly in the passive) To captivate.
ENAMOURED adjective
  1. In love, amorous.

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