Cryptic crossword clue
Figaro, say, one captivated by attractive girl 5

The most common and most likely answer to this crossword clue is the 6 letter word DO-ALL

D
O
-
A
L
L

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The straight part
We know that "Figaro, say" is the straight/definition part of the clue. The straight part is often a synonym or definition, in this case figaro, say = do-all.
The cryptic/wordplay part
In cryptic crossword there's often an wordplay/cryptic part as well.
This part involves a more complex hint, such as an anagram, homophone, hidden word, etc.
Sadly, We don't have an explanation for this specific crossword clue yet.

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