The most common and most likely answer to this crossword clue is the 9 letter word CACOETHES
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The straight part
We know that "Intense longing" is the straight/definition part of the clue. The straight part is often a synonym or definition, in this case intense longing = cacoethes.The cryptic/wordplay part
In cryptic crossword there's often an wordplay/cryptic part as well.This part involves a more complex hint, such as an anagram, homophone, hidden word, etc.
Sadly, We don't have an explanation for this specific crossword clue yet.
What does CACOETHES mean?
CACOETHES noun- Compulsion; mania.
- A bad quality or disposition in a disease; a malignant tumour or ulcer.