Cryptic crossword clue
Make a deep impression, bound by ties initially thought to be most vexatious 9

The most common and most likely answer to this crossword clue is the 9 letter word TETCHIEST

T
E
T
C
H
I
E
S
T

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The cryptic/wordplay part
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This part involves a more complex hint, such as an anagram, homophone, hidden word, etc.
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Crossword Answer definitions

TETCHIEST adjective
  1. Easily annoyed or irritated; peevish, testy or irascible.

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