The most common and most likely answer to this crossword clue is the 4 plus 2 letter word TIDY UP
I've seen this crossword clue in The Guardian
T
I
D
Y
U
P
Buddy explains!
The straight part
We know that "Make orderly" is the straight/definition part of the clue. The straight part is often a synonym or definition, in this case make orderly = tidy up.The cryptic/wordplay part
In cryptic crossword there's often an wordplay/cryptic part as well.This part involves a more complex hint, such as an anagram, homophone, hidden word, etc.
Sadly, We don't have an explanation for this specific crossword clue yet.
What does TIDY UP mean?
TIDY UP noun- An instance of something being tidied up.
- To make (something) more tidy.