Cryptic crossword clue
‘Samples’ torte, becomes most rotund the lion’s share

The most common and most likely answer to this crossword clue is the 7 letter word AMPLEST

A
M
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T

Buddy explains!

The straight part
We know that "most rotund" is the straight/definition part of the clue. The straight part is often a synonym or definition, in this case most rotund = amplest.
The cryptic/wordplay part
In cryptic crossword there's often an wordplay/cryptic part as well.
This part involves a more complex hint, such as an anagram, homophone, hidden word, etc.
Sadly, We don't have an explanation for this specific crossword clue yet.

What does AMPLEST mean?

AMPLEST adjective
  1. Large; great in size, extent, capacity, or bulk; for example spacious, roomy or widely extended.
  2. Fully sufficient; abundant; plenty
  3. Not contracted or brief; not concise; extended; diffusive

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